In this study, the elastomer cover, a new contact material, was developed to establish the customized ultrasonic measurement considering surface irregularities of stone cultural heritages. The cover exhibits high elastic force and wear resistance because it has tensile strength of 17㎫ and elongation of 625%. In addition, as a result of comparative experiments for the seven types according to transducers and contact materials including the elastomer cover, rock surface irregularities significantly affect attenuation of ultrasonic velocity. The phenomenon was more noticeable in the dabbed finish and direct transmission measurement rather than the chiseling finish and indirect transmission measurement. However, the Type F using the exponential transducer and elastomer cover showed stable P-wave velocity and high amplitude regardless of the surface irregularities. This because the elastomer cover sufficiently sticks to surface irregularities and removes pores between a transducer and a rock specimen. Therefore, the Type F should be used for the ultrasonic measurement of stone cultural heritages with surface irregularities.